Addressing high excitation conditions in time-resolved X-ray diffraction experiments and issues of biological relevance

JE Besaw, RJD Miller - Current Opinion in Structural Biology, 2023 - Elsevier
One of the most important fundamental questions connecting chemistry to biology is how
chemistry scales in complexity up to biological systems where there are innumerable …

Real-space subfemtosecond imaging of quantum electronic coherences in molecules

M Garg, A Martin-Jimenez, M Pisarra, Y Luo, F Martín… - Nature …, 2022 - nature.com
Tracking electron motion in molecules is the key to understanding and controlling chemical
transformations. Contemporary techniques in attosecond science are able to generate and …

High spatiotemporal resolution transmission electron microscopy and diffraction: Progress from subnanosecond laser-induced structural dynamics to femtosecond …

SA Aseyev, BN Mironov, DG Poydashev, EA Ryabov… - Nano Today, 2025 - Elsevier
The use of short photoelectron pulses, pioneered in the 1980s, opened up the possibility of
studying structural dynamics with high spatiotemporal resolution. The combination of nano …

Imaging purely nuclear quantum dynamics in molecules by combined x-ray and electron diffraction

H Yong, D Keefer, S Mukamel - Journal of the American Chemical …, 2022 - ACS Publications
Monitoring the motions of atoms and molecules in the course of chemical processes is a
central goal of femtochemistry. Optical spectroscopic signals are usually sensitive to …

Electronic Coherences in Molecules: The Projected Nuclear Quantum Momentum as a Hidden Agent

EV Arribas, NT Maitra - Physical review letters, 2024 - APS
Electronic coherences are key to understanding and controlling photoinduced molecular
transformations. We identify a crucial quantum-mechanical feature of electron-nuclear …

Attosecond charge migration in molecules imaged by combined x-ray and electron diffraction

H Yong, S Sun, B Gu, S Mukamel - Journal of the American …, 2022 - ACS Publications
We show how ultrafast gas-phase X-ray and electron diffraction signals can be combined to
generate real-space movies of charge migration dynamics in molecules. Charge migration …

Ultrafast imaging of molecular dynamics using ultrafast low-frequency lasers, X-ray free electron lasers, and electron pulses

M Zhang, Z Guo, X Mi, Z Li, Y Liu - The Journal of Physical …, 2022 - ACS Publications
The requirement of high space-time resolution and brightness is a great challenge for
imaging atomic motion and making molecular movies. Important breakthroughs in ultrabright …

Quantum state tomography of molecules by ultrafast diffraction

M Zhang, S Zhang, Y Xiong, H Zhang… - Nature …, 2021 - nature.com
Ultrafast electron diffraction and time-resolved serial crystallography are the basis of the
ongoing revolution in capturing at the atomic level of detail the structural dynamics of …

Anisotropic, nonthermal lattice disordering observed in photoexcited PbS quantum dots

KM Krawczyk, A Sarracini, PB Green… - The Journal of …, 2021 - ACS Publications
Given their nanoscale dimensions, colloidal semiconductor nanocrystals provide unique
systems for investigating the dynamics controlling surface chemistry and fundamental issues …

Time-resolved electron diffraction and microscopy of laser-induced processes in thin films

SA Aseyev, EA Ryabov, BN Mironov, IV Kochikov… - Chemical Physics …, 2022 - Elsevier
Using a compact diffractometer that was equipped with a pulsed electron source
synchronized with a femtosecond laser, a series of investigations of laser-stimulated …