Coherence in Chemistry: Foundations and Frontiers

JD Schultz, JL Yuly, EA Arsenault, K Parker… - Chemical …, 2024 - ACS Publications
Coherence refers to correlations in waves. Because matter has a wave-particle nature, it is
unsurprising that coherence has deep connections with the most contemporary issues in …

Phase-cycling and double-quantum two-dimensional electronic spectroscopy using a common-path birefringent interferometer

D Timmer, DC Lünemann, M Gittinger, A De Sio… - Optica, 2024 - opg.optica.org
Ultrafast spectroscopy provides unique access to the coherent dynamics of atomic,
molecular, and solid state quantum systems. A most powerful, yet experimentally …

A spectrometer design that eliminates incoherent mixing signals in 2D action spectroscopies

ZM Faitz, D Im, CJ Blackwell, MS Arnold… - The Journal of Chemical …, 2024 - pubs.aip.org
Action spectroscopies use a readout created by the action of light on the molecules or
material rather than optical absorption. Ultrafast 2D photocurrent and 2D fluorescence …

Cogwheel phase cycling in population-detected optical coherent multidimensional spectroscopy

A Jayachandran, S Mueller, T Brixner - The Journal of Chemical …, 2024 - pubs.aip.org
An integral procedure in every coherent multidimensional spectroscopy experiment is to
suppress undesired background signals. For that purpose, one can employ a particular …

Broadband rapid-scanning phase-modulated Fourier transform electronic spectroscopy

A Javed, J Lüttig, SE Sanders, F Sessa, AT Gardiner… - Optics …, 2024 - opg.optica.org
We present a phase-modulated approach for ultrabroadband Fourier transform electronic
spectroscopy. To overcome the bandwidth limitations and spatial chirp introduced by …

Light at the End of the Funnel: Fluorescence-Detected Two-Dimensional Electronic Spectroscopy to Probe Photosynthesis in Bacteria

A Javed - 2024 - deepblue.lib.umich.edu
Photosynthesis relies on solar energy absorption by the light-harvesting complexes and
ultrafast energy transfer to the reaction centers, where the excitation is converted into a …

One Step at a Time: Enhancing Fluorescence-Detected Two-Dimensional Electronic Spectroscopy

F Sessa - 2024 - deepblue.lib.umich.edu
Photosynthesis is the foundational biological process that converts light into chemical
energy. The initial steps of photosynthesis achieve near-unity quantum efficiency in …