Single-molecule nanomagnets

JR Friedman, MP Sarachik - Annu. Rev. Condens. Matter Phys., 2010 - annualreviews.org
Single-molecule magnets straddle the classical and quantum mechanical worlds, displaying
many fascinating phenomena. They may have important technological applications in …

Endohedral Metallofullerene as Molecular High Spin Qubit: Diverse Rabi Cycles in Gd2@C79N

Z Hu, BW Dong, Z Liu, JJ Liu, J Su, C Yu… - Journal of the …, 2018 - ACS Publications
An anisotropic high-spin qubit with long coherence time could scale the quantum system up.
It has been proposed that Grover's algorithm can be implemented in such systems …

Locking of electron spin coherence above 20 ms in natural silicon carbide

D Simin, H Kraus, A Sperlich, T Ohshima, GV Astakhov… - Physical Review B, 2017 - APS
We demonstrate that silicon carbide (SiC) with a natural isotope abundance can preserve a
coherent spin superposition in silicon vacancies over an unexpectedly long time exceeding …

Multiple quantum coherences from hyperfine transitions in a vanadium (IV) complex

JM Zadrozny, J Niklas, OG Poluektov… - Journal of the …, 2014 - ACS Publications
We report a vanadium complex in a nuclear-spin free ligand field that displays two key
properties for an ideal candidate qubit system: long coherence times that persist at high …

Magnetic strong coupling in a spin-photon system and transition to classical regime

I Chiorescu, N Groll, S Bertaina, T Mori… - Physical Review B …, 2010 - APS
We study the energy level structure of the Tavis-Cumming model applied to an ensemble of
independent magnetic spins s= 1/2 coupled to a variable number of photons. Rabi splittings …

Quantum computing with defects

L Gordon, JR Weber, JB Varley, A Janotti… - MRS bulletin, 2013 - cambridge.org
The successful development of quantum computers is dependent on identifying quantum
systems to function as qubits. Paramagnetic states of point defects in semiconductors or …

Magnetic coupling and single-ion anisotropy in surface-supported Mn-based metal–organic networks

L Giovanelli, A Savoyant, M Abel… - The Journal of …, 2014 - ACS Publications
The electronic and magnetic properties of Mn coordinated to 1, 2, 4, 5-tetracyanobenzene
(TCNB) in Mn–TCNB two-dimensional metal–ligand networks have been investigated by …

Coherent spin dynamics in a gadolinium-doped crystal

EI Baibekov, MR Gafurov, DG Zverev, IN Kurkin… - Physical Review B, 2017 - APS
We report the first observation of Rabi oscillations in the spin-7/2 ensemble of trivalent
gadolinium ions hosted in CaW O 4 single crystal. A number of transitions within the lowest …

Stable Mono‐Radical and Triplet Diradicals Based on Allylic Radical‐Embedded All‐Benzenoid Polycyclic Hydrocarbons

L Wang, W Niu, D Tian, T Jiao, L Zhang… - Angewandte …, 2025 - Wiley Online Library
High‐spin organic radicals are notable for their unique optical, electronic, and magnetic
properties, but synthesizing stable high‐spin systems is challenging due to their inherent …

Quantum simulations and experiments on Rabi oscillations of spin qubits: Intrinsic vs extrinsic damping

H De Raedt, B Barbara, S Miyashita, K Michielsen… - Physical Review B …, 2012 - APS
Electron paramagnetic resonance experiments show that the decay of Rabi oscillations of
ensembles of spin qubits depends noticeably on the microwave power, and more precisely …